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논문 해외 국제전문학술지(SCI급) Keeping it Simple: Free-Standing, Flexible Cathodic Electrodes for High Rate, Long Cycling Lithium Batteries

연구성과 설명 사진
  • 학술지 구분 국제전문학술지(SCI급)
  • 게재년월 2022-10
  • 저자명 Isheunesu Phiri, Jungmin Kim, Carlos Tafara Mpupuni, Kennedy Ssendagire, Jeong-Tae Kim, Yongmin Lee, and Sun-Yul Ryou
  • 학술지명 ACS Applied Energy Materials
  • 발행처명 American Chemical Society
  • 발행국가 해외
  • 논문언어 외국어
  • 전체저자수 7
  • 논문 다운로드 링크(외부) https://pubs.acs.org/doi/full/10.1021/acsaem.2c02211
  • 연구분야 공학 > 화학공학

논문 초록 (Abstract)

The manufacturing of flexible electronics requires flexible batteries. However, the development of high-performance flexible batteries has been rather slow. A majority of the available techniques are impractical and too expensive for industrial applications because of the type of equipment needed for preparing these flexible electrodes. Therefore, in this study, we developed a simple approach for fabricating free-standing flexible cathodic electrodes. The process involves the slurry casting of a well-dispersed electrode mixture comprising the active material, carbon fibers, polymer, plasticizer, and lithium salts. By adjusting the weight ratios, we realized the best trade-off between flexibility and specific capacity. The prepared free-standing flexible cathodic electrodes of lithium manganese oxide exhibited remarkably long cycling performance over 5000 cycles at 10 C versus Li metal anode with a coulombic efficiency (C.E.) > 99% The pouch cell also had excellent cycling performance of over 500 cycles at 5C with a C.E. > 99%. This method is simple and uses current battery production line equipment without the need for new specialized equipment. This could be cost-effective and efficient for manufacturing freestanding electrodes.